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Is there a natural 2-category of simplicial sets?
There is a fully faithful functor from the category of all small categories to the category of simplicial sets. The motivation for the question is that it might be more natural to consider the "collection" of all small categories as a 2-category.
I'm not sure what you're asking for. The most natural "2-category of simplicial sets" is obtained by enriching over itself and considering its image through the functor induced by the right adjoint of the nerve. This eventually leads to [[infinity-cosmos]] and all that.
it might be more natural to consider the "collection" of all small categories as a 2-category.
in what context are you talking about?
Thanks! I don't really know what you mean by "context".